The most difficult part is creating/extracting the textures (frames/fonts/etc) needed. Once the textures are in a WoW friendly format/dimensions (either Blizzard's .blp or .tga with an alpha channel, in a dimension that is any combo of powers of 2 such as 16, 32, 64, 128, 256, 512).
Then using existing mods such as Stuf or oUF (for the Unit Frames) and kgPanels (for other attaching to other frames) you can build your Borderlands themed UI. If you use Stuf you do not need any knowledge of Lua.
As the previous poster mentioned it's Lua not LUA. It's a word that is Brazilian in origin from the Portuguese word for "moon". It's not an acronym (like what NASA or the military loves to use).
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